Rapid single-particle chemical imaging of nanoplastics by SRS microscopy (Record no. 54996)

MARC details
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fixed length control field 02842nam a2200301Ia 4500
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control field MX-MdCICY
005 - DATE AND TIME OF LATEST TRANSACTION
control field 20250625162457.0
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Transcribing agency CICY
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Classification number (OCLC) (R) ; Classification number, CALL (RLIN) (NR) B-20916
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245 10 - TITLE STATEMENT
Title Rapid single-particle chemical imaging of nanoplastics by SRS microscopy
490 0# - SERIES STATEMENT
Volume/sequential designation Proceedings of the National Academy of Sciences, 121(3), p. e2300582121, 2024
520 3# - SUMMARY, ETC.
Summary, etc. Plastics are now omnipresent in our daily lives. The existence of microplastics (1 µm to 5 mm in length)and possibly even nanoplastics (<1 ?m)has recently raised health concerns. In particular, nanoplastics are believed to be more toxic since their smaller size renders them much more amenable, compared to microplastics, to enter the human body. However, detecting nanoplastics imposes tremendous analytical challenges on both the nano-level sensitivity and the plastic-identifying specificity, leading to a knowledge gap in this mysterious nanoworld surrounding us. To address these challenges, we developed a hyperspectral stimulated Raman scattering (SRS)imaging platform with an automated plastic identification algorithm that allows micro-nano plastic analysis at the single-particle level with high chemical specificity and throughput. We first validated the sensitivity enhancement of the narrow band of SRS to enable high-speed single nanoplastic detection below 100 nm. We then devised a data-driven spectral matching algorithm to address spectral identification challenges imposed by sensitive narrow-band hyperspectral imaging and achieve robust determination of common plastic polymers. With the established technique, we studied the micro-nano plastics from bottled water as a model system. We successfully detected and identified nanoplastics from major plastic types. Micro-nano plastics concentrations were estimated to be about 2.4 ± 1.3 × 105 particles per liter of bottled water, about 90 percent of which are nanoplastics. This is orders of magnitude more than the microplastic abundance reported previously in bottled water. High-throughput single-particle counting revealed extraordinary particle heterogeneity and nonorthogonality between plastic composition and morphologies; the resulting multidimensional profiling sheds light on the science of nanoplastics.
650 14 - SUBJECT ADDED ENTRY--TOPICAL TERM
Topical term or geographic name entry element RAMAN IMAGING
650 14 - SUBJECT ADDED ENTRY--TOPICAL TERM
Topical term or geographic name entry element STIMULATED RAMAN SCATTERING
650 14 - SUBJECT ADDED ENTRY--TOPICAL TERM
Topical term or geographic name entry element NANOPLASTICS
650 14 - SUBJECT ADDED ENTRY--TOPICAL TERM
Topical term or geographic name entry element OPTICAL MICROSCOPY
650 14 - SUBJECT ADDED ENTRY--TOPICAL TERM
Topical term or geographic name entry element SINGLE PARTICLE ANALYSIS
700 12 - ADDED ENTRY--PERSONAL NAME
Personal name Qian, N.
700 12 - ADDED ENTRY--PERSONAL NAME
Personal name Gao, X.
700 12 - ADDED ENTRY--PERSONAL NAME
Personal name Lang, X.
700 12 - ADDED ENTRY--PERSONAL NAME
Personal name Deng, H.
700 12 - ADDED ENTRY--PERSONAL NAME
Personal name Bratu, T. M.
700 12 - ADDED ENTRY--PERSONAL NAME
Personal name Chen, Q.
700 12 - ADDED ENTRY--PERSONAL NAME
Personal name Min, W.
856 40 - ELECTRONIC LOCATION AND ACCESS
Uniform Resource Identifier <a href="https://drive.google.com/file/d/1rJJ0dta7GOF7sTrkoPs5tDmsVMQ3k9ao/view?usp=drivesdk">https://drive.google.com/file/d/1rJJ0dta7GOF7sTrkoPs5tDmsVMQ3k9ao/view?usp=drivesdk</a>
Public note Para ver el documento ingresa a Google con tu cuenta: @cicy.edu.mx
942 ## - ADDED ENTRY ELEMENTS (KOHA)
Source of classification or shelving scheme Clasificación local
Koha item type Documentos solicitados
Holdings
Lost status Source of classification or shelving scheme Damaged status Not for loan Collection Home library Current library Shelving location Date acquired Total checkouts Full call number Date last seen Price effective from Koha item type
  Clasificación local     Ref1 CICY CICY Documento préstamo interbibliotecario 25.06.2025   B-20916 25.06.2025 25.06.2025 Documentos solicitados