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Co-catalytic effect of nickel in the electro-oxidation of ethanol on binary Pt-Sn electrocatalysts

Tipo de material: TextoTextoSeries ; ElectroChemistry Communications, 7(4), p.365-369, 2005Trabajos contenidos:
  • Spinace, E.V
  • Linardi, M
  • Oliveira Neto, A
Tema(s): Recursos en línea: Resumen: PtSn/C electrocatalysts with Pt:Sn molar ratios of 75:25, 50:50 and 25:75 and PtSnNi/C electrocatalyst with a Pt:Sn:Ni molar ratio of 50:40:10 were prepared by the alcohol-reduction process using ethylene glycol as solvent and reducing agent. The electrocatalysts were characterized by EDX, XRD and cyclic voltammetry. The electro-oxidation of ethanol was studied by cyclic voltammetry and chronoamperometry using the thin porous coating technique. PtSnNi/C electrocatalyst showed a superior performance compared to PtSn/C electrocatalysts in the potential range of interest for direct ethanol fuel cell.
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PtSn/C electrocatalysts with Pt:Sn molar ratios of 75:25, 50:50 and 25:75 and PtSnNi/C electrocatalyst with a Pt:Sn:Ni molar ratio of 50:40:10 were prepared by the alcohol-reduction process using ethylene glycol as solvent and reducing agent. The electrocatalysts were characterized by EDX, XRD and cyclic voltammetry. The electro-oxidation of ethanol was studied by cyclic voltammetry and chronoamperometry using the thin porous coating technique. PtSnNi/C electrocatalyst showed a superior performance compared to PtSn/C electrocatalysts in the potential range of interest for direct ethanol fuel cell.

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