Thermoplastic starch plasticized by an ionic liquid
Tipo de material:
TextoSeries ; Carbohydrate Polymers, 82(2), p.256-263, 2010Trabajos contenidos: - Sankri, A
- Arhaliass, A
- Dez, I
- Gaumont, A.C
- Grohens, Y
- Lourdin, D
- Pillin, I
- Pillin, I
- Leroy , E
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Thermoplastic starch (TPS)plasticized by 1-butyl-3-methylimidazolium chloride ([BMIM]Cl)was obtained by melt processing. The resulting electrically conductive TPS samples were less hygroscopic than glycerol plasticized TPS samples. Despite this lower water uptake, [BMIM]Cl seems to be intrinsically a more efficient plasticizer of starch. [BMIM]Cl plasticized TPS samples show a much higher elongation at break in the rubbery state than the glycerol plasticized TPS samples. Their unusually low rubbery Young's modulus for thermoplastic starch (0.5 MPa)suggests a strong reduction of hydrogen bonds between the starch chains due to the presence of the ionic liquid. A detailed IR spectroscopy analysis supports this interpretation.
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