Investigation of Factors Influencing the Chemoenzymatic Synthesis of Block Copolymers
Tipo de material:
TextoSeries ; Macromolecules, 38, p.4220-4225, 2005Trabajos contenidos: - De Geus, M
- Peeters, J
- Wolffs, M
- Hermans, T
- Palmans, A.R.A
- Koning, C.E
- Heise, A
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The chemoenzymatic synthesis of block copolymers from a bifunctional initiator using enzymatic ring-opening polymerization (eROP)and ATRP in two consecutive steps was investigated. First, a polycaprolactone (PCL)macroinitiator was obtained via an enzymatic ring-opening polymerization initiated by the bifunctional initiator. By carefully managing the water activity in the system, the amount of PCL not initiated by the bifunctional initiator was reduced to <5
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