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245 1 0 _aDevelopment of a sequential supercritical fluid extraction method for the analysis of nitrated and oxygenated derivatives of polycyclic aromatic hydrocarbons in urban aerosols
490 0 _vJournal of Chromatography A, 1010(2), p.141-151, 2003
520 3 _aA two-step supercritical fluid extraction (SFE)method has been developed for the analysis of oxygenated and nitrated polycyclic aromatic hydrocarbons (oxy- and nitro-PAHs, respectively)present in urban aerosol samples. The proposed SFE procedure first involves an extraction step using pure CO in order to remove the less polar compounds from the matrix and 2 a second consecutive step using toluene-modified CO . The oxy- and nitro-PAHs are obtained in the second step. Parameters 2 affecting both collection efficiencies and the selective extraction of oxy- and nitro-PAHs in the second SFE step were optimised. Analysis of the extracts was performed using gas chromatography with electron-capture detection and coupled to mass spectrometry. The proposed SFE method was compared with a conventional extraction technique such as onication and good agreement in the results was obtained. Nevertheless, clean up of sonication extracts was needed, whereas no purification was necessary for SFE extracts. The SFE method was applied to the analysis of oxy- and nitro-PAHs in urban aerosol samples and 9-fluorenone, 9,10-anthraquinone, 2-methyl-9,10-anthraquinone, benzanthrone, benz[a]anthracene-7,12- 23 dione and 1-nitropyrene were identified at concentrations ranging between 15 and 364 pg m .
650 1 4 _aAIR ANALYSIS
650 1 4 _aAEROSOLS
650 1 4 _aSUPERCRITICAL FLUID EXTRACTION
650 1 4 _aENVIRONMENTAL ANALYSIS
650 1 4 _aPOLYNUCLEAR AROMATIC HYDROCARBONS
650 1 4 _aNITRATED
650 1 4 _aPOLYNUCLEAR AROMATIC HYDROCARBONS
650 1 4 _aOXYGENATED
700 1 2 _aCastells, P.
700 1 2 _aSantos, F.J.
700 1 2 _aGalceran, M.T.
856 4 0 _uhttps://drive.google.com/file/d/1y6nG8CVkimTKtWPukgXe_3TmdcH5EWQX/view?usp=drivesdk
_zPara ver el documento ingresa a Google con tu cuenta: @cicy.edu.mx
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