000 02227nam a2200337Ia 4500
003 MX-MdCICY
005 20250625160148.0
040 _cCICY
090 _aB-16296
245 1 0 _aSynthesis of ZSM-5 zeolite with small crystal size and its catalytic performance for ethylene oligomerization
490 0 _vZeolites, 14(8), p.643-649, 1994
520 3 _aZSM-5 zeolites of SiO2 Al2O3 = 25 with a small crystal size were synthesized under various conditions in order to clarify a relationship between external surface area and catalytic performance, especially lifetime, for the oligomerization of ethylene to higher hydrocarbons of the gasoline range. The measurement of the external surface area, XRD patterns, and FTi.r. spectra of the resulting ZSM-5 zeolites suggested that their crystal grains were very fine. The shapes and sizes of the primary grains of the ZSM-5 zeolites were observed by means of a scanning electron microscopy with a magnification of 300,000. The crystal sizes were in the range of 30-50 nm. In the oligomerization of ethylene, a proton-type zeolite that was synthesized under a high molar ratio of OH SiO2 showed both high ethylene conversion and high gasoline range selectivity for three times longer on-stream time than those of other zeolites. The external surface area of the zeolite was also three times greater than those of other zeolites, which indicated that the lifetime of ZSM-5 zeolite in the oligomerization of ethylene depended on the external surface area or crystal size.
650 1 4 _aCATALYST SELECTIVITY
650 1 4 _aCRYSTAL STRUCTURE
650 1 4 _aCRYSTALLIZATION
650 1 4 _aCRYSTALS
650 1 4 _aETHYLENE
650 1 4 _aGRAIN SIZE AND SHAPE
650 1 4 _aHYDROCARBONS
650 1 4 _aSCANNING ELECTRON MICROSCOPY
650 1 4 _aSURFACE MEASUREMENT
650 1 4 _aSYNTHESIS (CHEMICAL)
700 1 2 _aYamamura, M.
700 1 2 _aChaki, K.
700 1 2 _aWakatsuki, T.
700 1 2 _aOkado, H.
700 1 2 _aFujimoto, K.
856 4 0 _uhttps://drive.google.com/file/d/1KXoGJXQmGDcpK7QmYrRoMD0BVXKNWKsY/view?usp=drivesdk
_zPara ver el documento ingresa a Google con tu cuenta: @cicy.edu.mx
942 _2Loc
_cREF1
008 250602s9999 xx |||||s2 |||| ||und|d
999 _c50470
_d50470