000 01820nam a2200241Ia 4500
003 MX-MdCICY
005 20250626083335.0
040 _cCICY
090 _aB-21599
245 1 0 _aPeriodate oxidation of chitosans with different chemical compositions
490 0 _aCarbohydrate Research, 340(4), p.679-684, 2005
500 _aArtículo
520 3 _aPeriodate oxidation of chitosans with different chemical compositions were investigated by determining the consumption of periodate consumed, and the amount of ammonia and formaldehyde liberated during the reaction. Oxidised chitosans were further characterised by size-exclusion chromatography with online multi-angle light scattering (SEC-MALLS) to obtain the molecular weight distributions, and by elemental analysis to obtain the N/C ratio. Chitosans became only partially oxidised by periodate, reaching degrees of oxidation around 0.5, when oxidising with excess periodate. Overconsumption of periodate is attributed to the extensive depolymerisation, which occurs concomitantly with the oxidation, thereby exposing novel reducing and non-reducing ends which consume additional periodate. Both the rate and extent of overoxidation, and the rate of depolymerisation decreased with increasing FA. A chitosan-specific degradation mechanism is probably involved in the depolymerisation in addition to the general free-radical-mediated degradation.
650 1 4 _aSEC-MALLS
650 1 4 _aFREE RADICALS
650 1 4 _aDEPOLYMERISATION
650 1 4 _aDIALDEHYDE
700 1 2 _aVold, I. M.
700 1 2 _aChristensen, B. E.
856 4 0 _uhttps://drive.google.com/file/d/1bYnuZupvvPNequyvQiPSXFOvZjZIPWmp/view?usp=drive_link
_zPara ver el documento ingresa a Google con tu cuenta: @cicy.edu.mx
942 _2Loc
_cREF1
008 250602s9999 xx |||||s2 |||| ||und|d
999 _c55667
_d55667